Boron-Functionalized Graphene Oxide-Organic Frameworks for Highly Efficient CO2 Capture

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dc.authoridWu, Kevin/0000-0003-0590-1396
dc.authoridKaneti, Yusuf Valentino/0000-0003-2433-7305
dc.authoridSarkar, Shuranjan/0000-0002-7760-9784
dc.authoridAlshehri, Saad/0000-0002-4990-6183
dc.authoridYamauchi, Yusuke/0000-0001-7854-927X
dc.authoridHOSSAIN, MD Shahriar/0000-0002-7291-9281
dc.authoridHaque, Enamul/0000-0002-2155-4382
dc.contributor.authorHaque, Enamul
dc.contributor.authorIslam, Md. Monirul
dc.contributor.authorPourazadi, Ehsan
dc.contributor.authorSarkar, Shuranjan
dc.contributor.authorHarris, Andrew T.
dc.contributor.authorMinett, Andrew I.
dc.contributor.authorYanmaz, Ekrem
dc.date.accessioned2024-09-11T19:50:04Z
dc.date.available2024-09-11T19:50:04Z
dc.date.issued2017
dc.departmentİstanbul Gelişim Üniversitesien_US
dc.description.abstractThe capture and storage of CO2 have been suggested as an effective strategy to reduce the global emissions of greenhouse gases. Hence, in recent years, many studies have been carried out to develop highly efficient materials for capturing CO2. Until today, different types of porous materials, such as zeolites, porous carbons, N/ Bdoped porous carbons or metal-organic frameworks (MOFs), have been studied for CO2 capture. Herein, the CO2 capture performance of new hybrid materials, graphene-organic frameworks (GOFs) is described. The GOFs were synthesized under mild conditions through a solvothermal process using graphene oxide (GO) as a starting material and benzene 1,4-diboronic acid as an organic linker. Interestingly, the obtained GOF shows a high surface area (506 m(2)g(-1)) which is around 11 times higher than that of GO (46 m(2)g(-1)), indicating that the organic modification on the GO surface is an effective way of preparing a porous structure using GO. Our synthetic approach is quite simple, facile, and fast, compared with many other approaches reported previously. The synthesized GOF exhibits a very large CO2 capacity of 4.95 mmol g(-1) at 298K (1 bar), which is higher those of other porous materials or carbon-based materials, along with an excellent CO2/N-2 selectivity of 48.8.en_US
dc.description.sponsorshipInternational Scientific Partnership Program (ISPP) at King Saud University (KSU) [ISPP-0024]en_US
dc.description.sponsorshipThe authors extend their appreciation to the International Scientific Partnership Program (ISPP) at King Saud University (KSU) for funding this research work through ISPP-0024.en_US
dc.identifier.doi10.1002/asia.201601442
dc.identifier.endpage288en_US
dc.identifier.issn1861-4728
dc.identifier.issn1861-471X
dc.identifier.issue3en_US
dc.identifier.pmid27943602en_US
dc.identifier.scopus2-s2.0-85010878207en_US
dc.identifier.startpage283en_US
dc.identifier.urihttps://doi.org/10.1002/asia.201601442
dc.identifier.urihttps://hdl.handle.net/11363/7550
dc.identifier.volume12en_US
dc.identifier.wosWOS:000393436000002en_US
dc.identifier.wosqualityQ2en_US
dc.indekslendigikaynakWeb of Scienceen_US
dc.language.isoenen_US
dc.publisherWiley-V C H Verlag Gmbhen_US
dc.relation.ispartofChemistry-An Asian Journalen_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.rightsinfo:eu-repo/semantics/closedAccessen_US
dc.snmz20240903_Gen_US
dc.subjectboronen_US
dc.subjectcarbon dioxide fixationen_US
dc.subjectgrapheneen_US
dc.subjectmesoporous materialsen_US
dc.titleBoron-Functionalized Graphene Oxide-Organic Frameworks for Highly Efficient CO2 Captureen_US
dc.typeArticleen_US

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